Return of naturally sourced Pb to Atlantic surface waters
Identifieur interne : 000011 ( Main/Exploration ); précédent : 000010; suivant : 000012Return of naturally sourced Pb to Atlantic surface waters
Auteurs : Luke Bridgestock [Royaume-Uni] ; Tina Van De Flierdt [Royaume-Uni] ; Mark Rehk Mper [Royaume-Uni] ; Maxence Paul [Royaume-Uni] ; Rob Middag [Nouvelle-Zélande, États-Unis] ; Angela Milne [Royaume-Uni] ; Maeve C. Lohan [Royaume-Uni] ; Alex R. Baker [Royaume-Uni] ; Rosie Chance [Royaume-Uni] ; Roulin Khondoker [Royaume-Uni] ; Stanislav Strekopytov [Royaume-Uni] ; Emma Humphreys-Williams [Royaume-Uni] ; Eric P. Achterberg [Allemagne] ; Micha J. A. Rijkenberg [Pays-Bas] ; Loes J. A. Gerringa [Pays-Bas] ; Hein J. W. De Baar [Pays-Bas]Source :
- Nature Communications [ 2041-1723 ] ; 2016.
Abstract
Anthropogenic emissions completely overwhelmed natural marine lead (Pb) sources during the past century, predominantly due to leaded petrol usage. Here, based on Pb isotope measurements, we reassess the importance of natural and anthropogenic Pb sources to the tropical North Atlantic following the nearly complete global cessation of leaded petrol use. Significant proportions of up to 30–50% of natural Pb, derived from mineral dust, are observed in Atlantic surface waters, reflecting the success of the global effort to reduce anthropogenic Pb emissions. The observation of mineral dust derived Pb in surface waters is governed by the elevated atmospheric mineral dust concentration of the North African dust plume and the dominance of dry deposition for the atmospheric aerosol flux to surface waters. Given these specific regional conditions, emissions from anthropogenic activities will remain the dominant global marine Pb source, even in the absence of leaded petrol combustion.
Url:
DOI: 10.1038/ncomms12921
PubMed: 27678297
PubMed Central: 5052796
Affiliations:
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Lohan</name><affiliation wicri:level="1"><nlm:aff id="a5"><institution>Ocean and Earth Sciences, National Oceanography Centre Southampton, University of Southampton</institution>, Southampton SO14 3ZH,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Baker, Alex R" sort="Baker, Alex R" uniqKey="Baker A" first="Alex R." last="Baker">Alex R. Baker</name><affiliation wicri:level="1"><nlm:aff id="a6"><institution>School of Environmental Sciences, University of East Anglia</institution>, Norwich NR4 7TJ,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Chance, Rosie" sort="Chance, Rosie" uniqKey="Chance R" first="Rosie" last="Chance">Rosie Chance</name><affiliation wicri:level="1"><nlm:aff id="a6"><institution>School of Environmental Sciences, University of East Anglia</institution>, Norwich NR4 7TJ,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Khondoker, Roulin" sort="Khondoker, Roulin" uniqKey="Khondoker R" first="Roulin" last="Khondoker">Roulin Khondoker</name><affiliation wicri:level="1"><nlm:aff id="a1"><institution>Department of Earth Science and Engineering, Imperial College London</institution>, London SW7 2AZ,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Strekopytov, Stanislav" sort="Strekopytov, Stanislav" uniqKey="Strekopytov S" first="Stanislav" last="Strekopytov">Stanislav Strekopytov</name><affiliation wicri:level="1"><nlm:aff id="a7"><institution>Image and Analysis Centre, Natural History Museum</institution>, London SW7 5BD,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Humphreys Williams, Emma" sort="Humphreys Williams, Emma" uniqKey="Humphreys Williams E" first="Emma" last="Humphreys-Williams">Emma Humphreys-Williams</name><affiliation wicri:level="1"><nlm:aff id="a7"><institution>Image and Analysis Centre, Natural History Museum</institution>, London SW7 5BD,<country>UK</country></nlm:aff><country xml:lang="fr">Royaume-Uni</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Achterberg, Eric P" sort="Achterberg, Eric P" uniqKey="Achterberg E" first="Eric P." last="Achterberg">Eric P. Achterberg</name><affiliation wicri:level="1"><nlm:aff id="a8"><institution>Geomar-Helmholtz Centre for Ocean Research</institution>, Kiel 24148,<country>Germany</country></nlm:aff><country xml:lang="fr">Allemagne</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Rijkenberg, Micha J A" sort="Rijkenberg, Micha J A" uniqKey="Rijkenberg M" first="Micha J. A." last="Rijkenberg">Micha J. A. Rijkenberg</name><affiliation wicri:level="1"><nlm:aff id="a9"><institution>Department of Ocean Systems (OCS), NIOZ Royal Netherlands Institute for Sea Research, and Utrecht University</institution>, P.O. Box 59, 1790 AB Den Burg, Texel,<country>The Netherlands</country></nlm:aff><country xml:lang="fr">Pays-Bas</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="Gerringa, Loes J A" sort="Gerringa, Loes J A" uniqKey="Gerringa L" first="Loes J. A." last="Gerringa">Loes J. A. Gerringa</name><affiliation wicri:level="1"><nlm:aff id="a9"><institution>Department of Ocean Systems (OCS), NIOZ Royal Netherlands Institute for Sea Research, and Utrecht University</institution>, P.O. Box 59, 1790 AB Den Burg, Texel,<country>The Netherlands</country></nlm:aff><country xml:lang="fr">Pays-Bas</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author><author><name sortKey="De Baar, Hein J W" sort="De Baar, Hein J W" uniqKey="De Baar H" first="Hein J. W." last="De Baar">Hein J. W. De Baar</name><affiliation wicri:level="1"><nlm:aff id="a9"><institution>Department of Ocean Systems (OCS), NIOZ Royal Netherlands Institute for Sea Research, and Utrecht University</institution>, P.O. Box 59, 1790 AB Den Burg, Texel,<country>The Netherlands</country></nlm:aff><country xml:lang="fr">Pays-Bas</country><wicri:regionArea># see nlm:aff country strict</wicri:regionArea></affiliation></author></analytic><series><title level="j">Nature Communications</title><idno type="eISSN">2041-1723</idno><imprint><date when="2016">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en"><p>Anthropogenic emissions completely overwhelmed natural marine lead (Pb) sources during the past century, predominantly due to leaded petrol usage. Here, based on Pb isotope measurements, we reassess the importance of natural and anthropogenic Pb sources to the tropical North Atlantic following the nearly complete global cessation of leaded petrol use. Significant proportions of up to 30–50% of natural Pb, derived from mineral dust, are observed in Atlantic surface waters, reflecting the success of the global effort to reduce anthropogenic Pb emissions. The observation of mineral dust derived Pb in surface waters is governed by the elevated atmospheric mineral dust concentration of the North African dust plume and the dominance of dry deposition for the atmospheric aerosol flux to surface waters. Given these specific regional conditions, emissions from anthropogenic activities will remain the dominant global marine Pb source, even in the absence of leaded petrol combustion.</p></div></front><back><div1 type="bibliography"><listBibl><biblStruct><analytic><author><name sortKey="Nriagu, J O" uniqKey="Nriagu J">J. O. Nriagu</name></author><author><name sortKey="Pacyna, J M" uniqKey="Pacyna J">J. M. Pacyna</name></author></analytic></biblStruct><biblStruct><analytic><author><name sortKey="Boyle, E A" uniqKey="Boyle E">E. A. 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Achterberg</name></noRegion></country><country name="Pays-Bas"><noRegion><name sortKey="Rijkenberg, Micha J A" sort="Rijkenberg, Micha J A" uniqKey="Rijkenberg M" first="Micha J. A." last="Rijkenberg">Micha J. A. Rijkenberg</name></noRegion><name sortKey="De Baar, Hein J W" sort="De Baar, Hein J W" uniqKey="De Baar H" first="Hein J. W." last="De Baar">Hein J. W. De Baar</name><name sortKey="Gerringa, Loes J A" sort="Gerringa, Loes J A" uniqKey="Gerringa L" first="Loes J. A." last="Gerringa">Loes J. A. Gerringa</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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